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Theoretical study of heterogeneous reaction kinetics: A comparison between microcalorimetric and thermogravimetric curves

Abstract : In the kinetic theories of Bodenstein or Semenov the expression for the rate of a chemical reaction with several elementary stages can be expressed by different physical parameters. If two experimental methods are used, one method of necessity being microcalorimetry to measure the thermal flux produced by the reaction, it is possible to distinguish a pure kinetics case from a mixed one. The two-method technique has been verified by a study of the oxidation of niobium.
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https://hal-emse.ccsd.cnrs.fr/emse-00433799
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Submitted on : Friday, November 20, 2009 - 10:54:45 AM
Last modification on : Wednesday, June 24, 2020 - 4:18:18 PM

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René Lalauze, Alain Souchon, Michel Soustelle. Theoretical study of heterogeneous reaction kinetics: A comparison between microcalorimetric and thermogravimetric curves. Oxidation of Metals, Springer Verlag, 1976, 10 (2), pp.105-111. ⟨10.1007/BF00614240⟩. ⟨emse-00433799⟩

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